top of page

Exploring 2D quantum materials with ultralow wavenumber Raman spectroscopy in an Argon glovebox

2D quantum materials exhibit unique electronic, optical, and magnetic properties, promising advancements for photonics, quantum computing, and sensing applications.



Exploring intriguing many-body physics in 2D quantum materials


Using ultralow wavenumber Raman spectroscopy to investigate critical quantum phenomena in 2D materials, researchers at QPalmLab aim to understand and measure quantum properties such as lattice vibrations (phonons), electronic structures influenced by stacking order and strain, spin excitations (magnons), charge density wave phenomena, and amplitudon modes in 2D quantum materials:


  • Stacking order and strain: Tuning stacking configurations and strain in layered materials can directly influence electronic band structures and optical responses, allowing for custom-engineered quantum states and devices.

  • Charge density waves (CDWs): Detailed exploration of CDWs reveals insight into superconducting phases and electronic phase transitions that reveal correlated electron behaviours that are crucial for advancing quantum computing and sensing solutions.

  • Magnon excitations and spin dynamics: Probing magnon dynamics allows for the exploration of spin-based phenomena at the quantum level, enabling advancements in ultra-low power quantum memory, logic, and data storage applications.


Limitations of traditional Raman spectroscopy


Raman spectroscopy provides sensitive, non-destructive insights into vibrational modes, electronic structures, and spin dynamics of these 2D quantum materials. However, traditional Raman techniques often suffer from environmental interference, sample degradation under laser excitation, and gas ionization that can introduce noise and distort spectra — significantly reducing the accuracy and reproducibility of experimental results. The research conducted at QPalmLab addresses these limitations by using an ultralow wavenumber Raman spectroscopy system integrated into an argon-filled glovebox. A key component of this setup is the Skylark 320 NX CW DPSS UV laser.


Features of the Skylark 320 NX ultraviolet laser for Raman spectroscopy


The Skylark 320 NX operating at 320 nm is central to this Raman spectroscopy setup — selected for its power and wavelength stability, narrow linewidth, and spectral purity.


  • Ultra-stable output: Consistent power and wavelength enables clear, reproducible Raman measurements of 2D quantum materials.

  • Narrow linewidth: The narrow spectral linewidth significantly enhances spectral resolution, allowing the precise capture of subtle quantum properties.

  • Reduced ionization effects: Spectral purity paired with narrow linewidth minimises gas ionization — reducing noise and distortion in Raman spectra.



Stable and reliable investigation of 2D quantum materials using an argon-filled glovebox and ultralow wavenumber Raman spectroscopy


The argon environment suppresses rotational signals from nitrogen (N₂) and oxygen (O₂), enhancing the clarity of spectral data. Argon also protects delicate 2D samples from degradation caused by high-power laser exposure. Additionally, the inert argon environment significantly reduces the gas ionization issues associated with UV lasers — ensuring more stable and consistent experimental conditions. This setup improves experimental reliability and leverages the spectral quality of the laser systems, facilitating clearer investigations into the quantum properties of 2D materials.



Exploring 2D quantum materials with ultralow wavenumber Raman spectroscopy - research poster

FOR FURTHER INFORMATION

Dr. Shao-Yu Chen




Conclusion


The integration of ultralow wavenumber Raman spectroscopy within an argon-filled glovebox significantly enhances the reliability and accuracy of quantum material research. By mitigating common challenges faced in Raman spectroscopy, this method enables deeper and clearer investigations of quantum phenomena, supporting advances in quantum technologies and device applications.

 
 
bottom of page